High-performance liquid chromatography determination of ketone bodies in human plasma by precolumn derivatization with p-nitrobenzene diazonium fluoroborate

Anal Biochem. 2009 Jan 1;384(1):145-50. doi: 10.1016/j.ab.2008.09.017. Epub 2008 Sep 17.

Abstract

We developed and validated a sensitive and convenient high-performance liquid chromatography (HPLC) method for the specific determination of ketone bodies (acetoacetate and D-3-hydroxybutyrate) in human plasma. p-Nitrobenzene diazonium fluoroborate (diazo reagent) was used as a precolumn derivatization agent, and 3-(2-hydroxyphenyl) propionic acid was used as an internal standard. After the reaction, excess diazo reagent and plasma proteins were removed by passing through a solid-phase cartridge (C(18)). The derivatives retained on the cartridge were eluted with methanol, introduced into the HPLC system, and then detected with UV at 380 nm. A calibration curve for acetoacetate standard solution with a 20-microl injection volume showed good linearity in the range of 1 to 400 microM with a 0.9997 correlation coefficient. For the determination of D-3-hydroxybutyrate, it was converted to acetoacetate before reaction with the diazo reagent by an enzymatic coupling method using D-3-hydroxybutyrate dehydrogenase and lactate dehydrogenase. A calibration curve for D-3-hydroxybutyrate standard solution also showed good linearity in the range of 1.5 to 2000 microM with a 0.9988 correlation coefficient. Analytical recoveries of acetoacetate and D-3-hydroxybutyrate in human plasma were satisfactory. The method was successfully applied to samples from diabetic patients, and results were consistent with those obtained using the thio-NAD enzymatic cycling method used in clinical laboratories.

Publication types

  • Comparative Study
  • Evaluation Study

MeSH terms

  • Calibration
  • Chromatography, High Pressure Liquid / methods*
  • Diazonium Compounds / chemistry*
  • Humans
  • Ketone Bodies / blood*
  • Phenylpropionates / chemistry

Substances

  • 3-(2-hydroxyphenyl)propionic acid
  • Diazonium Compounds
  • Ketone Bodies
  • Phenylpropionates
  • 4-nitrobenzene diazonium tetrafluoroborate