Characterization of pyruvate kinase of Trypanosoma brucei and its role in the regulation of carbohydrate metabolism

Mol Biochem Parasitol. 1991 Jul;47(1):19-29. doi: 10.1016/0166-6851(91)90144-u.

Abstract

Pyruvate kinase from Trypanosoma brucei is a labile enzyme, losing its activity within several hours. In mixtures containing 50 mM triethanolamine buffer, pH 7.2, 25% glycerol and 0.5 mM inorganic phosphate the enzyme remained active and could be purified to homogeneity with a specific activity of 417 units mg-1 and a yield of 65%. The enzyme has an activation energy of 31.9 kJ mol-1. Magnesium and potassium ions are essential for activity. Cobalt or manganese ions replace Mg2+ but this leads to a decrease in maximal velocity. Potassium ions can be substituted by ammonium ions, while sodium ions behave as a competitive inhibitor with respect to both K+ and NH4+. All metal ions studied displayed sigmoidal kinetics. The enzyme is activated, with decreasing efficiency by fructose 2-phosphorothioate 6-phosphate, fructose 2,6-bisphosphate, fructose 1,6-bisphosphate and glucose 1,6-bisphosphate. They all display hyperbolic kinetics. Glycerate 2,3-bisphosphate, glyceraldehyde 3-phosphate, CoASAc, oxalate, AMP, ADP, and ATP inhibit the enzyme. At substrate saturation PK was activated by Pi up to a concentration of 0.8 mM. At higher Pi concentrations the enzyme is inhibited. The enzyme is unaffected by most amino acids, only phenylalanine stimulates and tyrosine inhibits.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acids / pharmacology
  • Animals
  • Anions / pharmacology
  • Carbohydrate Metabolism*
  • Cations / pharmacology
  • Enzyme Stability / drug effects
  • Erythrocytes / drug effects
  • Erythrocytes / parasitology
  • Kinetics
  • Phosphates / pharmacology
  • Pyruvate Kinase / isolation & purification
  • Pyruvate Kinase / metabolism
  • Pyruvate Kinase / physiology*
  • Temperature
  • Trypanosoma brucei brucei / drug effects
  • Trypanosoma brucei brucei / enzymology*
  • Trypanosoma brucei brucei / growth & development

Substances

  • Amino Acids
  • Anions
  • Cations
  • Phosphates
  • Pyruvate Kinase