Abstract
Three new coumarins containing a C(10) terpenoid side chain, clauslactones R - T (1 - 3), together with 14 known coumarins (4 - 17) and 11 known carbazole alkaloids (18 - 28), were isolated from the leaves and stems of Clausena excavata. Their structures were established by detailed spectroscopic analyses. Furthermore, the stereochemistry of 1 was confirmed by single-crystal X-ray diffraction analysis, which was the first example among coumarins with a C(10) terpenoid side chain. Additionally, compounds 22 and 27 were found to show moderate topoisomerase II inhibitory effects at 50 microM.
Publication types
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Research Support, Non-U.S. Gov't
MeSH terms
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Clausena / chemistry*
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Coumarins / chemistry*
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Coumarins / isolation & purification
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Coumarins / pharmacology
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Enzyme Inhibitors / chemistry
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Enzyme Inhibitors / isolation & purification
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Enzyme Inhibitors / pharmacology
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Magnetic Resonance Spectroscopy
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Molecular Conformation
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Plant Leaves / chemistry
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Plant Stems / chemistry
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Spectrometry, Mass, Electrospray Ionization
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Spectrophotometry, Infrared
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Spectrophotometry, Ultraviolet
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Structure-Activity Relationship
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Topoisomerase II Inhibitors
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X-Ray Diffraction
Substances
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Coumarins
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Enzyme Inhibitors
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Topoisomerase II Inhibitors