Abstract
The O-antigen structure of Shigella dysenteriae type 2 was reinvestigated using chemical modifications along with high-resolution 2D (1)H and (13)C NMR spectroscopy. The O-antigen was found to contain a pyruvic acid acetal, which was overlooked in an early study, and the following revised structure of the pentasaccharide repeating unit was established: where approximately 70% GlcNAc residues bear an O-acetyl group at position 3. The O-antigen of Escherichia coli O112ac was found to have the same carbohydrate structure but to lack O-acetylation.
Publication types
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Research Support, Non-U.S. Gov't
MeSH terms
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Carbohydrate Sequence
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Chromatography, Gas
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Escherichia coli / chemistry*
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Hydrolysis
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Lipopolysaccharides / chemistry
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Lipopolysaccharides / isolation & purification
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Magnetic Resonance Spectroscopy
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Molecular Sequence Data
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Monosaccharides / analysis
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O Antigens / chemistry*
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O Antigens / isolation & purification
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Pyruvates / analysis
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Shigella dysenteriae / chemistry*
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Trifluoroacetic Acid / analysis
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Trifluoroacetic Acid / chemistry
Substances
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Lipopolysaccharides
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Monosaccharides
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O Antigens
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Pyruvates
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pyruvic acid acetal
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Trifluoroacetic Acid