In vivo studies on the antileishmanial activity of buparvaquone and its prodrugs

J Antimicrob Chemother. 2007 Oct;60(4):802-10. doi: 10.1093/jac/dkm303. Epub 2007 Aug 21.

Abstract

Objectives: The efficacy of different formulations of the naphthoquinone buparvaquone and two phosphate prodrugs in in vivo models of both visceral and cutaneous leishmaniasis is described.

Methods: Several topical formulations of buparvaquone containing acceptable excipients were tested in vivo against Leishmania major cutaneous lesions in BALB/c mice. In vivo studies against Leishmania donovani investigated whether the prodrugs had improved efficacy when compared with buparvaquone.

Results: Both a hydrous gel and water-in-oil emulsion of buparvaquone significantly reduced cutaneous parasite burden (P < 0.05, 22 days post-infection) and lesion size, compared with the untreated control (P < 0.0001, 16 days post-infection). The prodrug 3-phosphonooxymethyl-buparvaquone was formulated into an anhydrous gel and this also significantly reduced parasite burden and lesion size (P < 0.0001, 16 days post-infection). Histology confirmed this efficacy. In the visceral model, both prodrugs were significantly more effective at reducing liver parasite burden than the parent drug, buparvaquone. Buparvaquone-3-phosphate was shown to be the most effective antileishmanial (P = 0.0003, 50 mg buparvaquone molar equivalent/kg/day five times), reducing the liver parasite burden by approximately 34% when compared with the untreated control.

Conclusions: The introduction of a topical formulation, such as buparvaquone (or its prodrug), would be a significant advance for the treatment of simple cutaneous lesions. In particular, the avoidance of the parenteral antimonials would greatly increase patient compliance and reduce treatment costs.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Antiprotozoal Agents / administration & dosage
  • Antiprotozoal Agents / therapeutic use*
  • Chemistry, Pharmaceutical
  • Female
  • Leishmania donovani / drug effects*
  • Leishmania major / drug effects*
  • Leishmaniasis, Cutaneous / drug therapy
  • Leishmaniasis, Visceral / drug therapy
  • Liver / parasitology
  • Mice
  • Mice, Inbred BALB C
  • Naphthoquinones / administration & dosage
  • Naphthoquinones / therapeutic use*
  • Prodrugs / administration & dosage
  • Prodrugs / therapeutic use*
  • Skin / parasitology
  • Skin / pathology

Substances

  • Antiprotozoal Agents
  • Naphthoquinones
  • Prodrugs
  • buparvaquone