New insights into NIS-promoted aminocyclization. Synthesis of decahydroquinolines from 2-allylcyclohexylamines

Org Lett. 2007 Jul 5;9(14):2633-6. doi: 10.1021/ol070770g. Epub 2007 Jun 6.

Abstract

Bishomoallylic secondary amines embodying the 2-allyl-N-benzylcyclohexylamine unit react with NIS to undergo cyclization through 6-endo processes in either the cis or trans series. Nevertheless, when the resulting cis-3-iododecahydroquinolines are treated with Al2O3, the exo derivatives evolve into octahydroindoles and the endo derivatives keep the same backbone, the configuration being retained in the generated alcohols.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amines / chemical synthesis*
  • Cyclization
  • Cyclohexylamines / chemistry*
  • Indicators and Reagents
  • Nickel / chemistry*
  • Quinolines / chemical synthesis*

Substances

  • Amines
  • Cyclohexylamines
  • Indicators and Reagents
  • Quinolines
  • Nickel
  • nickel sulfide