Purification by ozonolysis of (18)O enriched water after cyclotron irradiation and the utilization of the purified water for the production of [18F]-FDG (2-deoxy-2-[18F]-fluoro-d-glucose)

Appl Radiat Isot. 2007 Jul;65(7):831-5. doi: 10.1016/j.apradiso.2007.03.003. Epub 2007 Mar 19.

Abstract

The high cost of virgin (18)O-enriched water has forced many researchers to study methods to purify and recycle enriched water after the first irradiation for the production of radiopharmaceuticals. In our study, [(18)O]H(2)O was purified by ozonolysis and distillation. Analyses showed a large decrease in impurities after this treatment. The purification procedure was carried out after the production of 94 batches of [18F]-FDG, which were manufactured using a GE Minitrace cyclotron and a GE Mx TracerLab synthesizer. Saturation yields after bombardment, using virgin and re-purified water were, respectively, 2864+/-204MBq/muA and 2727+/-167MBq/muA, a decrease of 5.5%. The decrease in [18F]-FDG yield, from 67.2+/-0.7% to 65.5+/-0.9%, can be ascribed to the irradiation step only.

MeSH terms

  • Cyclotrons
  • Fluorodeoxyglucose F18 / chemistry*
  • Oxygen Isotopes / chemistry*
  • Radiopharmaceuticals / chemistry*
  • Water / chemistry*

Substances

  • Oxygen Isotopes
  • Radiopharmaceuticals
  • Water
  • Fluorodeoxyglucose F18