Evaluation of thioglycosides of Kdo as glycosyl donors

Carbohydr Res. 2007 Feb 26;342(3-4):631-7. doi: 10.1016/j.carres.2006.08.021. Epub 2006 Oct 9.

Abstract

The use of Kdo thioglycosides as glycosyl donors using DMTST, IBr/AgOTf and NIS/AgOTf as promoters has been evaluated. Activation at low temperature allowed to escape the formation of 2,3-glycal byproducts to give glycosides in high yield and with good beta-anomeric selectivity. The use of diethyl ether as solvent and (especially) isopropylidene acetals as protecting groups improved the alpha-anomeric selectivity. NIS/AgOTf as promoter surprisingly yielded the 3-iodo-product via the glycal intermediate.

Publication types

  • Evaluation Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Disulfides / chemistry
  • Glycosylation
  • Mesylates / chemistry
  • Sugar Acids / chemistry*
  • Thioglycosides / chemistry*

Substances

  • Disulfides
  • Mesylates
  • Sugar Acids
  • Thioglycosides
  • dimethyl(methylthio)sulfonium
  • trifluoromethanesulfonic acid
  • 3-deoxy-manno-oct-2-ulopyranosonic acid