Structural elucidation of the O-antigenic polysaccharide from enterohemorrhagic (EHEC) Escherichia coli O48:H21

Carbohydr Res. 2006 Nov 6;341(15):2543-9. doi: 10.1016/j.carres.2006.08.008. Epub 2006 Sep 1.

Abstract

The structure of the antigenic O-polysaccharide (O-PS) of the lipopolysaccharide (LPS) produced by the enterohemorrhagic strain of Escherichia coli O48:H21 (EHEC) has been elucidated. The O-PS obtained by mild acid hydrolysis of the LPS had [alpha]D +95 (water) and was composed of L-rhamnose (L-Rha), D-galactose (D-Gal), 2-amino-2-deoxy-D-glucose (D-GlcN), 2-amino-2-deoxy-D-galactose (D-GalN), and D-galacturonic acid (D-GalA) (1:1:1:1:1). From the results of methylation analysis, mass spectrometry, 2D NMR, and DOC-PAGE, the O-PS was shown to be a high molecular mass polymer of a repeating pentasaccharide unit having the structure: [structure: see text]. The D-Gal pA non-reducing end groups in the O-PS were partially O-acetylated (approximately 30%) at the O-2 and O-3 positions and the degree of acetylation was variable from batch to batch cell production.

MeSH terms

  • Carbohydrate Conformation
  • Carbohydrate Sequence
  • Chromatography, Gel
  • Escherichia coli O157 / chemistry*
  • Indicators and Reagents
  • Lipopolysaccharides / chemistry
  • Lipopolysaccharides / isolation & purification
  • Magnetic Resonance Spectroscopy
  • Models, Molecular
  • Molecular Sequence Data
  • O Antigens / chemistry*
  • Polysaccharides, Bacterial / chemistry*

Substances

  • Indicators and Reagents
  • Lipopolysaccharides
  • O Antigens
  • Polysaccharides, Bacterial