Torsional steering controls the stereoselectivity of epoxidation in the guanacastepene a synthesis

Org Lett. 2006 Apr 13;8(8):1513-6. doi: 10.1021/ol052862g.

Abstract

[reaction: see text] The stereoselectivity of the key epoxidation step in the synthesis of guanacastepene A is shown to be controlled by torsional steering. In this particular epoxidation reaction, the transition structure energetic difference is enhanced by the great asynchronicity of the forming C-O bonds that intensifies the torsional interactions.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Crystallography, X-Ray
  • Diterpenes / chemical synthesis
  • Diterpenes / chemistry
  • Models, Molecular
  • Molecular Conformation
  • Molecular Structure
  • Stereoisomerism

Substances

  • Diterpenes
  • guanacastepene