A triple diene-transmissive Diels-Alder strategy to build the quassinoid framework

Org Lett. 2005 Dec 8;7(25):5601-4. doi: 10.1021/ol0522236.

Abstract

[chemical reaction: see text]. An advanced intermediate to the highly oxygenated triterpene quassinoids was prepared in 14 steps from tetrahydrofuran. The key steps are three diene-transmissive Diels-Alder cycloadditions. Several features of this synthesis are noteworthy, including a successful Mitsunobu reaction on an allenylic alcohol, a rare [4 + 2] cycloaddition involving an enethiol ether dienophile, and complete control over all 10 chiral centers created.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cyclization
  • Furans / chemical synthesis
  • Furans / chemistry*
  • Molecular Structure
  • Oxidation-Reduction
  • Quassins / chemical synthesis*
  • Quassins / chemistry*

Substances

  • Furans
  • Quassins