Validation of 5 routine assays for serum free testosterone with a candidate reference measurement procedure based on ultrafiltration and isotope dilution-gas chromatography-mass spectrometry

Clin Biochem. 2005 Mar;38(3):253-61. doi: 10.1016/j.clinbiochem.2004.12.001.

Abstract

Background/method: The analytical validity of free testosterone (FTe) analog immunoassays is subject to much controversy. We revisited the validation of 4 analog assays and 1 FTe calculation procedure with a metrologically traceable reference measurement procedure (RMP) based on ultrafiltration and isotope dilution-mass spectrometry for direct measurement of Te in the ultrafiltrate. To this end, we performed split-sample measurements of 40 male sera.

Results: Deming regression showed that 3 of the immunoassays had moderate to good correlation (0.8474 < or = r < or = 0.9241) with the RMP; however, the slope was markedly below 1. The FTe calculation procedure was in good agreement with this result. The Sy/x values for all assays were higher than the combined imprecision values, which indicate their susceptibility to matrix-related effects.

Conclusions: The study demonstrated substantial differences in analytical quality of FTe assays; however, the results suggested that after extending the validation with a larger variety of samples, recalibration of some analog assays might be worth further investigation.

Publication types

  • Research Support, Non-U.S. Gov't
  • Validation Study

MeSH terms

  • Adult
  • Calibration
  • Carbon Isotopes
  • Gas Chromatography-Mass Spectrometry
  • Humans
  • Hypogonadism / diagnosis
  • Immunoassay / methods
  • Indicator Dilution Techniques
  • Male
  • Middle Aged
  • Reference Values
  • Reproducibility of Results
  • Sensitivity and Specificity
  • Testosterone / blood*
  • Ultrafiltration

Substances

  • Carbon Isotopes
  • Testosterone