Atrazine transformation using synthetic enzymes prepared by molecular imprinting

Org Biomol Chem. 2004 Sep 21;2(18):2563-6. doi: 10.1039/B407002J. Epub 2004 Aug 17.

Abstract

Atrazine imprinted synthetic polymers were prepared using a combination of methacrylic acid and 2-sulfoethyl methacrylate that bound and converted atrazine and other 6-chlorotriazine herbicides to less toxic compounds. A chloride at the 6-position of the triazines was converted to a methoxy group by the polymer in a methanol-containing solvent, where the imprinting effects enhanced the catalytic activity. Competitive inhibition of the atrazine methanolysis was observed in the presence of a structurally related binder, ametryn, suggesting that the catalytic reaction proceeded in the binding sites generated by the molecular imprinting process.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Atrazine / chemistry*
  • Binding Sites
  • Catalysis
  • Herbicides / chemistry*
  • Kinetics
  • Methacrylates / chemistry
  • Molecular Structure
  • Polymers / chemistry*

Substances

  • Herbicides
  • Methacrylates
  • Polymers
  • Atrazine