Temperature and cryoprotectant influence secondary quinone binding position in bacterial reaction centers

FEBS Lett. 2004 Jul 16;570(1-3):171-4. doi: 10.1016/j.febslet.2004.06.042.

Abstract

We have determined the first de novo position of the secondary quinone QB in the Rhodobacter sphaeroides reaction center (RC) using phases derived by the single wavelength anomalous dispersion method from crystals with selenomethionine substitution. We found that in frozen RC crystals, QB occupies primarily the proximal binding site. In contrast, our room temperature structure showed that QB is largely in the distal position. Both data sets were collected in dark-adapted conditions. We estimate that the occupancy of the QB site is 80% with a proximal: distal ratio of 4:1 in frozen RC crystals. We could not separate the effect of freezing from the effect of the cryoprotectants ethylene glycol or glycerol. These results could have far-reaching implications in structure/function studies of electron transfer in the acceptor quinone complex because the above are the most commonly used cryoprotectants in spectroscopic experiments.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Benzoquinones / chemistry
  • Binding Sites
  • Cryoprotective Agents / pharmacology*
  • Crystallography, X-Ray
  • Electrons
  • Ethylene Glycol / chemistry
  • Ethylene Glycol / pharmacology
  • Glycerol / chemistry
  • Glycerol / pharmacology
  • Light
  • Models, Chemical
  • Phosphates / pharmacology
  • Photosynthetic Reaction Center Complex Proteins / chemistry*
  • Potassium Compounds / pharmacology
  • Protein Binding
  • Protein Conformation
  • Quinones / chemistry*
  • Rhodobacter sphaeroides / metabolism
  • Selenomethionine / chemistry
  • Temperature
  • X-Ray Diffraction

Substances

  • Benzoquinones
  • Cryoprotective Agents
  • Phosphates
  • Photosynthetic Reaction Center Complex Proteins
  • Potassium Compounds
  • Quinones
  • quinone
  • Selenomethionine
  • potassium phosphate
  • Ethylene Glycol
  • Glycerol