Functional identification of the gene locus (ncg12319 and characterization of catechol 1,2-dioxygenase in Corynebacterium glutamicum

Biotechnol Lett. 2004 Apr;26(7):575-80. doi: 10.1023/b:bile.0000021958.86258.08.

Abstract

Corynebacterium glutamicum assimilated phenol, benzoate, 4-hydroxybenzoate p-cresol and 3,4-dihydroxybenzoate. Ring cleavage was by catechol 1,2-dioxygenase when phenol or benzoate was used and by protocatechuate 3,4-dioxygenase when the others were used as substrate. The locus ncg12319 of its genome was cloned and expressed in Escherichia coli. Enzyme assays showed that ncg12319 encodes a catechol 1,2-dioxygenase. This catechol 1,2-dioxygenase was purified and accepted catechol, 3-, or 4-methylcatechols, but not chlorinated catechols, as substrates. The optimal temperature and pH for catechol cleavage catalyzed by the enzyme were 30 degrees C and 9, respectively, and the Km and Vmax were determined to be 4.24 micromol l(-1) and 3.7 micromol l(-1) min(-1) mg(-1) protein, respectively.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Catechol 1,2-Dioxygenase
  • Chromosome Mapping*
  • Cloning, Molecular / methods
  • Corynebacterium / enzymology*
  • Corynebacterium / genetics*
  • Dioxygenases / chemistry*
  • Dioxygenases / genetics*
  • Dioxygenases / metabolism
  • Enzyme Activation
  • Enzyme Stability
  • Escherichia coli / enzymology
  • Escherichia coli / genetics
  • Gene Expression Profiling*
  • Molecular Sequence Data
  • Molecular Weight
  • Protein Conformation
  • Recombinant Proteins / chemistry
  • Recombinant Proteins / metabolism
  • Sequence Homology, Amino Acid

Substances

  • Recombinant Proteins
  • Dioxygenases
  • Catechol 1,2-Dioxygenase