Systemic and spinal analgesic activity of a delta-opioid-selective lanthionine enkephalin analog

J Pharmacol Exp Ther. 2003 Feb;304(2):827-32. doi: 10.1124/jpet.102.039750.

Abstract

A lanthionine enkephalin derivative, Tyr-c[D-Val(L)-Gly-Phe-D-Ala(L)]-OH (DV(L)(2)DA(L)(5)LanEnk), where Val(L) and Ala(L) denote the lanthionine amino acid ends linked via a monosulfide bridge to form the lanthionine structure, was synthesized. It was found to possess selectivity for and potency at the delta versus mu opioid receptor as defined by binding studies and by its respective activity on the mouse vas deferens compared with the guinea pig ileum. The agent produced a potent analgesia after intrathecal and intraperitoneal delivery with ED(50) values being, respectively, 0.19 mucrog and 0.49 mg/kg. The effects of the agent were reversed by the delta-selective antagonist naltrindole. These analgesic actions occurred at doses that had no effect upon general behavior or motor function. These results suggest a potent delta-preferring agent suitable for development as a systemic delta opioid analgesic.

Publication types

  • Comparative Study

MeSH terms

  • Alanine / analogs & derivatives*
  • Alanine / chemistry
  • Alanine / pharmacology*
  • Analgesics, Opioid / chemistry
  • Analgesics, Opioid / pharmacology*
  • Animals
  • Dose-Response Relationship, Drug
  • Enkephalin, D-Penicillamine (2,5)- / analogs & derivatives
  • Enkephalin, D-Penicillamine (2,5)- / pharmacology
  • Enkephalins / chemistry
  • Enkephalins / pharmacology*
  • Guinea Pigs
  • In Vitro Techniques
  • Male
  • Mice
  • Pain Measurement / drug effects
  • Pain Measurement / methods
  • Rats
  • Rats, Sprague-Dawley
  • Receptors, Opioid, delta / agonists
  • Receptors, Opioid, delta / physiology*
  • Spinal Cord / drug effects*
  • Spinal Cord / physiology
  • Sulfides

Substances

  • Analgesics, Opioid
  • Enkephalins
  • Receptors, Opioid, delta
  • Sulfides
  • tyrosyl-(valyl-glycyl-phenylalanyl-alanyl)-OH
  • Enkephalin, D-Penicillamine (2,5)-
  • lanthionine
  • Alanine