Sensitive and rapid liquid chromatography-tandem mass spectrometry method for the determination of stavudine in human plasma

J Chromatogr B Analyt Technol Biomed Life Sci. 2002 Jun 25;773(2):129-34. doi: 10.1016/s1570-0232(02)00136-8.

Abstract

A sensitive method for the determination of stavudine in plasma was developed, using high-performance liquid chromatographic separation with tandem mass spectrometric detection. The samples were extracted from plasma with Waters, Sep-Pak Vac, 100 mg, tC(18) solid-phase extraction (SPE) columns. Chromatography was performed on a Supelco Discovery C(18), 5 microm, 150 x 2 mm column with a mobile phase consisting of ammonium acetate (0.01 M)-acetonitrile-methanol (800:100:100, v/v/v) at a flow-rate of 0.3 ml/min. Detection was achieved by an Applied Biosystems API 2000 mass spectrometer (LC-MS-MS) set at unit resolution in the multiple reaction monitoring mode (MRM). Atmospheric pressure chemical ionization (APCI) was used for ion production. The mean recovery for stavudine was 94% with a lower limit of quantification set at 4 ng/ml. This assay method makes use of the increased sensitivity and selectivity of mass spectrometric (MS-MS) detection to allow for a more rapid (extraction and chromatography) and selective method for the determination of stavudine in human plasma than has previously been described.

MeSH terms

  • Chromatography, Liquid / methods*
  • Humans
  • Mass Spectrometry / methods*
  • Reverse Transcriptase Inhibitors / blood*
  • Reverse Transcriptase Inhibitors / pharmacokinetics
  • Sensitivity and Specificity
  • Stavudine / blood*
  • Stavudine / pharmacokinetics

Substances

  • Reverse Transcriptase Inhibitors
  • Stavudine