Determination of 17alpha-hydroxypregnenolone in human plasma by routine isotope dilution mass spectrometry using benchtop gas chromatography-mass selective detection

Steroids. 2001 Oct;66(10):759-62. doi: 10.1016/s0039-128x(01)00109-x.

Abstract

A first assay based on stable isotope dilution/gas chromatography-mass spectrometry has been developed for plasma 17alpha-hydroxypregnenolone, the leading marker of 3beta-hydroxysteroid dehydrogenase deficiency. Equilibration of plasma with internal standard was followed by solid phase extraction. After clean up using Sephadex LH-20 mini columns, heptafluorobutyrates were prepared as derivatives. Quantification was achieved by selected ion monitoring of m/z 467.0 (analyte) and m/z 471.0 (internal standard). 0.030 pmol of 17alpha-hydroxypregnenolone gave a signal to noise ratio of 3.7. Calibration plot was linear. Spiking experiments showed good accuracy with relative errors < 3.7%. Intraassay precision CV was 8.3% and interassay precision CV was 5.6%. Requiring small amounts of plasma, the rapid, convenient work up and the application of bench top GC/MS instrumentation proved our method suitable for routine clinical use in adults and children.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • 17-alpha-Hydroxypregnenolone / blood*
  • 3-Hydroxysteroid Dehydrogenases / deficiency
  • Adolescent
  • Adult
  • Child
  • Child, Preschool
  • Female
  • Gas Chromatography-Mass Spectrometry / methods
  • Humans
  • Infant
  • Infant, Newborn
  • Isotope Labeling
  • Male
  • Mass Spectrometry / methods*

Substances

  • 17-alpha-Hydroxypregnenolone
  • 3-Hydroxysteroid Dehydrogenases