Efficient biochemical engineering of cellular sialic acids using an unphysiological sialic acid precursor in cells lacking UDP-N-acetylglucosamine 2-epimerase

FEBS Lett. 2001 Aug 10;503(1):80-4. doi: 10.1016/s0014-5793(01)02701-6.

Abstract

Sialic acids comprise a family of terminal sugars essential for a variety of biological recognition systems. N-Propanoylmannosamine, an unphysiological sialic acid precursor, is taken up and metabolized by mammalian cells resulting in oligosaccharide-bound N-propanoylneuraminic acid. N-Propanoylmannosamine, applied to endogenously hyposialylated subclones of the myeloid leukemia HL60 and of the B-cell lymphoma BJA-B, both deficient in UDP-N-acetylglucosamine 2-epimerase, is efficiently metabolized to CMP-N-propanoylneuraminic acid resulting in up to 85% of glycoconjugate-associated sialic acids being unphysiological N-propanoylneuraminic acid. Thus, UDP-N-acetylglucosamine 2-epimerase-deficient cell lines provide an important experimental progress in engineering cells to display an almost homogeneous population of defined, structurally altered sialic acids.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Carbohydrate Epimerases / metabolism*
  • Cell Line
  • Cell Membrane / metabolism
  • Cytidine Monophosphate N-Acetylneuraminic Acid / chemistry
  • Cytidine Monophosphate N-Acetylneuraminic Acid / metabolism*
  • Escherichia coli Proteins*
  • Flow Cytometry
  • Humans
  • Neuraminic Acids / metabolism
  • Tumor Cells, Cultured

Substances

  • Escherichia coli Proteins
  • N-propanoylneuraminic acid
  • Neuraminic Acids
  • Cytidine Monophosphate N-Acetylneuraminic Acid
  • Carbohydrate Epimerases
  • UDP acetylglucosamine-2-epimerase
  • wecB protein, E coli