Reactive oxygen species from NAD(P)H:quinone oxidoreductase constitutively activate NF-kappaB in malignant melanoma cells

Am J Physiol Cell Physiol. 2001 Mar;280(3):C659-76. doi: 10.1152/ajpcell.2001.280.3.C659.

Abstract

The transcription factor nuclear factor-kappaB (NF-kappaB) is constitutively activated in malignancies from enhanced activity of inhibitor of NF-kappaB (IkappaB) kinase, with accelerated IkappaBalpha degradation. We studied whether redox signaling might stimulate these events. Cultured melanoma cells generated superoxide anions (O(2)(-)) without serum stimulation. O(2)(-) generation was reduced by the NAD(P)H:quinone oxidoreductase (NQO) inhibitor dicumarol and the quinone analog capsaicin, suggesting that electron transfer from NQO through a quinone-mediated pathway may be an important source of endogenous reactive oxygen species (ROS) in tumor cells. Treatment of malignant melanoma cells with the H(2)O(2) scavenger catalase, the sulfhydryl donor N-acetylcysteine, the glutathione peroxidase mimetic ebselen, or dicumarol decreased NF-kappaB activation. Catalase, N-acetylcysteine, ebselen, dicumarol, and capsaicin also inhibited growth of melanoma and other malignant cell lines. These results raise the possibility that ROS produced endogenously by mechanisms involving NQO can constitutively activate NF-kappaB in an autocrine fashion and suggest the potential for new antioxidant strategies for interruption of oxidant signaling of melanoma cell growth.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Antioxidants / pharmacology
  • Capsaicin / pharmacology
  • Cell Division / drug effects
  • Dicumarol / pharmacology
  • Enzyme Inhibitors / pharmacology
  • Humans
  • Melanoma / metabolism*
  • Melanoma / pathology
  • NADH, NADPH Oxidoreductases / metabolism*
  • NADP / physiology
  • NF-kappa B / drug effects
  • NF-kappa B / physiology*
  • Ploidies
  • Reactive Oxygen Species / physiology*
  • S Phase / drug effects
  • Tumor Cells, Cultured

Substances

  • Antioxidants
  • Enzyme Inhibitors
  • NF-kappa B
  • Reactive Oxygen Species
  • NADP
  • Dicumarol
  • NADH, NADPH Oxidoreductases
  • NAD(P)H plastoquinone oxidoreductase
  • Capsaicin