Fluorescence lifetime for on-the-fly multiplex detection of DNA restriction fragments in capillary electrophoresis

Anal Chem. 2000 Nov 1;72(21):5444-9. doi: 10.1021/ac000235t.

Abstract

This paper describes the first use of frequency-domain fluorescence lifetime for multiplex detection of DNA restriction fragments in capillary electrophoresis (CE). The fragments were labeled with monomeric intercalating dyes that can be excited by either the 488- or 514-nm line of an argon ion laser and have lifetimes in the range of 0.5-2.5 ns. We were able to achieve multiplex lifetime detection in the CE separation of a restriction fragment digest and a DNA size ladder in the same run, for fragments shorter than 700 bp. Different gel buffer systems, including a modified polyacrylamide gel and several tris-borate-EDTA/hydroxyethylcellulose (TBE/HEC) gels, were investigated for separation and detection of the dye-labeled DNA fragments. Best results for both electrophoretic resolution and lifetime detection were obtained using a gel containing 1% high molecular weight (90,000-105,000) HEC and 0.3% low molecular weight (24,000-27,000) HEC in TBE buffer.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • DNA / chemistry*
  • Electrophoresis, Capillary
  • Fluorescent Dyes
  • Indicators and Reagents
  • Intercalating Agents
  • Spectrophotometry, Ultraviolet

Substances

  • Fluorescent Dyes
  • Indicators and Reagents
  • Intercalating Agents
  • DNA