Stereoselective measurement of E- and Z-doxepin and its N-desmethyl and hydroxylated metabolites by gas chromatography-mass spectrometry

J Chromatogr B Biomed Sci Appl. 1999 Dec 24;736(1-2):201-8. doi: 10.1016/s0378-4347(99)00458-2.

Abstract

A stereoselective method of analysis of the antidepressant drug doxepin (DOX, an 85:15% mixture of E-Z stereoisomers), its principal metabolites E- and Z-N-desmethyldoxepin (desDOX) and ring-hydroxylated metabolites in microsomal incubation mixtures is described. DOX and its metabolites were extracted from alkalinised incubation mixtures by either: 9:1 hexane-propan-2-ol (method 1) or 1:1 hexane-dichloromethane (method 2), derivatised with trifluoroacetic anhydride and analysed by GC-MS with selected ion monitoring. Both methods were suitable for the analysis of individual desDOX isomers as indicated by correlation coefficients of > or = 0.999 for calibration curves constructed between 50 and 2500 nM, and good within-day precision at 125 nM (C.V. < or = 14%) and 1000 nM (C.V. < or = 8%). Method 1, however, was unsuitable for the analysis of ring-hydroxylated metabolites of DOX, whereas the hydroxylated metabolites of E-DOX and E-desDOX (generated in situ) were extracted by method 2 with a C.V. of ca. 13%. This is the first assay method that permits the simultaneous measurement of desDOX and hydroxylated metabolites of DOX in microsomal mixtures.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antidepressive Agents, Tricyclic / analysis*
  • Calibration
  • Doxepin / analogs & derivatives
  • Doxepin / analysis*
  • Doxepin / metabolism
  • Gas Chromatography-Mass Spectrometry / methods*
  • Gas Chromatography-Mass Spectrometry / standards
  • Humans
  • Hydrogen-Ion Concentration
  • Hydroxylation
  • Microsomes, Liver / chemistry
  • Microsomes, Liver / metabolism
  • Nortriptyline
  • Sensitivity and Specificity
  • Stereoisomerism

Substances

  • Antidepressive Agents, Tricyclic
  • Doxepin
  • Nortriptyline
  • desmethyldoxepin