Crystal structure of the secreted form of antigen 85C reveals potential targets for mycobacterial drugs and vaccines

Nat Struct Biol. 2000 Feb;7(2):141-6. doi: 10.1038/72413.

Abstract

The antigen 85 (ag85) complex, composed of three proteins (ag85A, B and C), is a major protein component of the Mycobacterium tuberculosis cell wall. Each protein possesses a mycolyltransferase activity required for the biogenesis of trehalose dimycolate (cord factor), a dominant structure necessary for maintaining cell wall integrity. The crystal structure of recombinant ag85C from M. tuberculosis, refined to a resolution of 1.5 A, reveals an alpha/beta-hydrolase polypeptide fold, and a catalytic triad formed by Ser 124, Glu 228 and His 260. ag85C complexed with a covalent inhibitor implicates residues Leu 40 and Met 125 as components of the oxyanion hole. A hydrophobic pocket and tunnel extending 21 A into the core of the protein indicates the location of a probable trehalose monomycolate binding site. Also, a large region of conserved surface residues among ag85A, B and C is a probable site for the interaction of ag85 proteins with human fibronectin.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Acyltransferases*
  • Amino Acid Sequence
  • Antigens, Bacterial / chemistry*
  • Antigens, Bacterial / drug effects
  • Antigens, Bacterial / immunology
  • Antigens, Bacterial / metabolism*
  • Antitubercular Agents / chemistry
  • Binding Sites
  • Catalytic Domain
  • Cell Wall / metabolism
  • Cord Factors / metabolism
  • Crystallography, X-Ray
  • Drug Design
  • Fibronectins / metabolism*
  • Humans
  • Models, Molecular
  • Molecular Sequence Data
  • Mycobacterium tuberculosis
  • Organophosphates / chemistry
  • Organophosphates / metabolism
  • Protein Conformation
  • Recombinant Proteins / chemistry
  • Recombinant Proteins / drug effects
  • Recombinant Proteins / immunology
  • Recombinant Proteins / metabolism

Substances

  • Antigens, Bacterial
  • Antitubercular Agents
  • Cord Factors
  • Fibronectins
  • Organophosphates
  • Recombinant Proteins
  • diethyl phosphate
  • Acyltransferases
  • antigen 85C, Mycobacterium tuberculosis

Associated data

  • PDB/1DQY
  • PDB/1DQZ