A rapid reusable fiber optic biosensor for detecting cocaine metabolites in urine

J Anal Toxicol. 1999 Oct;23(6):460-7. doi: 10.1093/jat/23.6.460.

Abstract

Analyte 2000, a four-channel fiber optic biosensor (FOB), was used for analysis of cocaine and its metabolites (COC) in human urine using a competitive fluorescence immunoassay. Binding of antibenzoylecgonine monoclonal antibody (mAb) to the casein-benzoylecgonine Ag-coated, tapered optical fibers was inhibited by COC. Bound mAb, which inversely correlated with COC concentration, was quantitated by fluorescence produced by evanescent excitation of bound cyanine dye-tagged antimouse antibody (CY5-Ab). The effective concentration range of benzoylecgonine (BE) for inhibiting the fluorescent signals was 0.75-50 ng/mL, with IC50 of 9.0 ng/mL. This FOB had similar affinities for BE, cocaine, and cocaethylene, but very low affinities for ecgonine and ecgonine methyl ester. A sensitivity of 100% and a specificity of 96% were achieved when 54 human urine specimens were analyzed by FOB (cutoff, 300 ng/mL COC) and GC-MS (cutoff, 150 ng/mL BE). All results were in agreement except for one positive FOB result with a GC-MS BE concentration of 148 ng/mL. In addition, regeneration and reuse of the fiber for multiple analyses were performed successfully with no carryover from specimens containing high COC concentrations to specimens containing low COC concentrations.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Antibodies, Monoclonal / immunology
  • Biosensing Techniques / methods*
  • Cocaine / analogs & derivatives*
  • Cocaine / analysis
  • Cocaine / chemistry
  • Cocaine / metabolism
  • Cocaine / urine*
  • Dopamine Uptake Inhibitors / analysis
  • Fiber Optic Technology / methods*
  • Fluorescence Polarization Immunoassay
  • Humans
  • Narcotics / analysis*
  • Narcotics / urine
  • Optical Fibers
  • Protein Binding
  • Reproducibility of Results
  • Sensitivity and Specificity
  • Urine / chemistry*

Substances

  • Antibodies, Monoclonal
  • Dopamine Uptake Inhibitors
  • Narcotics
  • benzoylecgonine
  • cocaethylene
  • Cocaine