A Germanium Zeotype Containing Intratunnel Transition Metal Complexes

Angew Chem Int Ed Engl. 1999 Aug;38(16):2436-2439. doi: 10.1002/(sici)1521-3773(19990816)38:16<2436::aid-anie2436>3.0.co;2-w.

Abstract

A new zeolite-type structure is adopted by (NH(4))(+)[M(NH(3))(2)](+)(Ge(9)O(19))(2-) (M=Cu, Ag; shown in the picture). These compounds are the first microporous germanates containing a transition metal complex inside their tunnels. The large separation between the metal centers and the unhindered access of reactants to these active sites through uniformly sized channels make these materials a good point of departure for designing new catalysts.