High-performance liquid chromatographic separation of the biotransformation products of oxaliplatin

J Chromatogr B Biomed Sci Appl. 1999 Mar 19;724(2):345-56. doi: 10.1016/s0378-4347(98)00565-9.

Abstract

A novel single reversed-phase HPLC system was developed for separating oxaliplatin and its biotransformation products formed in rat plasma. The major stable biotransformation products of oxaliplatin formed in rat plasma were identified as Pt(dach)(Cys)2, Pt(dach)(Met) and free dach. The minor biotransformation products Pt(dach)Cl2, Pt(dach)(GSH) and Pt(dach)(GSH)2 could also be resolved from other Pt-dach complexes. Among these biotransformation products, the identification of Pt(dach)(Met) was further confirmed by LC-ESI-MS, and the identification of Pt(dach)(Cys)2, Pt(dach)(GSH), Pt(dach)(GSH)2 and free dach was confirmed by atomic absorption and double isotope labeling. This HPLC technique should prove useful for separating and identifying the biotransformation products of Pt-dach drugs such as oxaliplatin, ormaplatin and Pt(dach)(mal) in biological fluids. This will allow a more complete characterization of the pharmacokinetics and biotransformations of these Pt-dach drugs, which should in turn lead to a better understanding of the mechanisms leading to their toxicity and efficacy.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Animals
  • Antineoplastic Agents / blood
  • Antineoplastic Agents / pharmacokinetics*
  • Biotransformation
  • Chromatography, High Pressure Liquid / methods*
  • Male
  • Mass Spectrometry
  • Organoplatinum Compounds / blood
  • Organoplatinum Compounds / pharmacokinetics*
  • Oxaliplatin
  • Rats
  • Rats, Wistar

Substances

  • Antineoplastic Agents
  • Organoplatinum Compounds
  • Oxaliplatin